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IDENTIFYING THE NEUROPHYSIOLOGICAL MECHANISMS UNDERLYING THE POTENTIAL THERAPEUTIC EFFECTS OF PSYCHEDELIC COMPOUNDS

Gavin P. Schmitz

UNC Libraries May 21, 2026 DOI: 10.17615/1vmn-e026 (opens in new tab)

Study at a glance

AI-extracted from the abstract
Characteristics Dissertation combining receptor pharmacology, genetic analysis, and electrophysiological studies Peer reviewed
Interventions Psilocin 25-CN-NBOH 2-bromo-LSD
Topics LSD
Keywords Neurophysiology Electrophysiology Posterior cingulate Hallucinogen Prefrontal cortex Population Infralimbic cortex Cognition Mechanism biology Premovement neuronal activity Pyramidal cell Local field potential Anterior cingulate cortex Mechanism of action
Key points All tested psychedelic compounds are agonists at the 5-HT2A serotonin receptor, and psilocin increases firing in prefrontal cortex 5-HT2A neurons via a 5-HT2A- and Gαq-dependent mechanism, while the non-hallucinogenic LSD analog 2-bromo-LSD reduces firing through a different mechanism.

Abstract

Psychedelics are seeing renewed interest due to their potential as therapeutic tools; however, despite promising clinical findings, the underlying signaling mechanisms and brain-region specific effects of psychedelics remain unclear. This dissertation first describes a comprehensive study aimed at understanding the on and off-target actions of ~40 diverse psychedelic substances representing each class of psychedelic compounds: the tryptamine, phenethylamine, and lysergamide groups. Significant serotonergic, dopaminergic, and adrenergic agonism activities are described, but all tested psychedelic compounds are found to be agonists at the 5-HT2A serotonin receptor. This dissertation next describes the effects of the seven most common naturally occurring sequence variations in the human 5-HT2AR gene on the signaling of four commonly used psychedelic drugs. The 5-HT2AR is robustly enriched in layer V pyramidal (L5p) neurons in both rodent and human cortices, and positron emission tomography studies in humans have shown that psilocin’s psychedelic effects correlate with 5-HT2AR occupancy in the prefrontal cortex (PFC)[1]. As part of this dissertation, electrophysiological studies identify a population of 5-HT2AR neurons in the prelimbic (PrL)/anterior cingulate (ACC) region of the PFC. Psilocin and the 5-HT2AR-prefering compound 25-CN-NBOH increased firing in these neurons through a mechanism that is both 5-HT2AR and Gq dependent. Finally, in contrast, the non-hallucinogenic lysergic acid diethylamide (LSD) analog 2-bromo-LSD (2-Br-LSD) reduces firing in both 5-HT2AR neurons and non-5-HT2AR neurons in a non-5-HT2AR dependent manner. Together, these data provide robust insights into psychedelic drug action by examining the receptor pharmacology of psychedelic compounds, the impact of genetic variance on 5-HT2AR signaling, the neurophysiological effects of psychedelics in the PFC, and the differential effects of a non-hallucinogenic LSD analog on PFC cellular physiology and behavior.

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