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Synthesis and Pharmacological Evaluation of Ring-Methylated Derivatives of 3,4-(Methylenedioxy)amphetamine (MDA)

Matthew Parker, Danuta Marona‐lewicka, Deborah M. Kurrasch, Alexander T. Shulgin, David E. Nichols

Journal of Medicinal Chemistry February 24, 1998 DOI: 10.1021/jm9705925 (opens in new tab)

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AI-extracted from the abstract
Characteristics In vivo and in vitro pharmacological study Peer reviewed
Population Rat brain synaptosomal preparations and live rats
Topics Serotonin
Keywords Methylenedioxy Pharmacology Hallucinogen Amphetamine In vivo Stereochemistry Antidepressant Monoamine neurotransmitter Amitriptyline Biochemistry Receptor Dopamine Hippocampus Organic chemistry
Citations 25
Key points The 2-methyl and 5-methyl derivatives of MDA are more potent and selective than MDA in releasing serotonin and are among the most potent serotonin-releasing compounds known.

Abstract

The three isomeric ring-methylated derivatives of the well-known hallucinogen and entactogen MDA (1a) were synthesized and evaluated for pharmacological activity as monoamine-releasing agents and as serotonin agonists. The 2-methyl derivative 2a and the 5-methyl derivative 2b were found to be more potent and more selective than the parent compound in inhibiting [3H]-serotonin accumulation in rat brain synaptosomal preparations. Their activity in vivo was confirmed in rats trained to discriminate serotonin-releasing agents and hallucinogens from saline. The results indicate that compounds 2a,b are among the most potent 5-HT-releasing compounds known and show promise as lead compounds in the search for antidepressant drugs that release serotonin rather than inhibit its uptake.

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